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J. Vac. Sci. Technol. A 28, 1371 (2010); http://dx.doi.org/10.1116/1.3498716 (6 pages)

Isolation of exchange- and spin-orbit-driven effects via manipulation of the axis of quantization a

a This article is based on material presented at the 57th Symposium of the American Vacuum Society.
Takashi Komesu1, G. D. Waddill1, S.-W. Yu2, M. T. Butterfield2, and J. G. Tobin2

1Department of Physics, Missouri University of Science and Technology, Rolla, Missouri 65401
2Lawrence Livermore National Laboratory, LLNS-LLC, Livermore, California 94550

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(Published online 13 October 2010)

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Double polarization photoelectron spectroscopy using circularly polarized x-rays and true spin detection has been performed using the 2p core levels of ultrathin films of Fe and Co. This includes both the separation into magnetization- and spin-specific spectra and an analysis of the polarization, asymmetry, and related quantities. It is shown how to selectively manipulate the manifestation of exchange- and spin-orbit effects simply by choosing different axes of quantization. Furthermore, the underlying simplicity of the results can be confirmed by comparison to a simple yet powerful single-electron picture.

© 2010 American Vacuum Society

ACKNOWLEDGMENTS

Lawrence Livermore National Laboratory is operated by Lawrence Livermore National Security, LLC, for the U.S. Department of Energy, National Nuclear Security Administration under Contract No. DE-AC52-07NA27344. This work was supported by the DOE Office of Science, Office of Basic Energy Science, Division of Materials Science and Engineering. The APS has been built and operated under funding from the Office of Basic Energy Science at DOE. We would like to thank the scientific and technical staff of Sector 4 of the Advanced Photon Source for their technical assistance in supporting this work. T.K. would like to thank Peter A. Dowben at University of Nebraska-Lincoln for valuable scientific discussions.

Article Outline

  1. INTRODUCTION
  2. EXPERIMENT
  3. DISCUSSION OF EXPERIMENTAL CONCEPT
  4. DISCUSSION OF EXPERIMENTAL RESULTS AND SPECTRAL ANALYSIS
    1. Ferromagnetically ordered Fe
    2. Magnetically disordered Co
  5. CONCLUSIONS

KEYWORDS and PACS

PACS

  • 71.70.Ej

    Spin-orbit coupling, Zeeman and Stark splitting, Jahn-Teller effect

  • 75.60.Ej

    Magnetization curves, hysteresis, Barkhausen and related effects

  • 79.60.-i

    Photoemission and photoelectron spectra

  • 75.70.Ak

    Magnetic properties of monolayers and thin films

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PUBLICATION DATA

ISSN

0734-2101 (print)  
1520-8559 (online)

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